We're going to take a look at some of the best villains on the PS3 that left the heroes in the dust. And he's not just all talk because, at the beginning of the game, he's already killed over a billion people. 5 Final Fantasy XIII-2Destined to FailFinal Fantasy XIII-2 has the best villain in the 3-game arc in the form of Caius Ballad. 3 Tales of BerseriaArtorius the BoldTales of Berseria is an awesome title in the Tales series with some great combat, a compelling story and arguably the best villain in the series. It's a wild premise and Zero is a compelling character in her own right, but the main villain steals the show.