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EN
Modular monomer precursor enables functional and biodegradable polyamino esters
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European Coatings
N-acylated poly(amino esters) (PAEs) synthesised via organocatalytic ring-opening polymerisation (ROP) are promising materials for functional and degradable applications.
A research team has now developed a universal monomer precursor for N-acylated 1,4-oxazepan-7-ones (OxPs) through a three-step synthesis, allowing the introduction of various functional groups.
Two novel oxidation-sensitive OxP monomers bearing a double bond or a sulphide group were designed, along with two monomers containing alkyl moieties.
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In addition, the (bio)degradability of the N-acylated PAEs was evaluated under mild enzymatic catalysis, in neutral phosphate-buffered saline solution and under accelerated conditions.
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