Results and DiscussionThe results demonstrated that the synthesized covalent organic nanosheets exhibited notable stability and tunable electronic properties. Overall, the study highlights the potential of these covalent organic nanosheets as versatile, high-performance battery electrodes. ConclusionThis study successfully introduces a robust strategy for synthesizing covalent organic nanosheets that combine adjustable electronic properties with unprecedented stability in sodium-ion batteries. The implications of this work extend across sodium-ion energy storage and closely related technologies, positioning covalent organic nanosheets as promising candidates for next-generation nano-engineered devices. Covalent Organic Nanosheets with a Tunable Electronic Structure to Achieve Unprecedented Stability and High-Performance in Sodium-Ion Batteries.